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(Keynote) Enabling High-Rate Lithium Metal Anodes By Tailored Structures and Interfaces

作者:E. Wachsman · 发表于:ECS Meeting Abstracts · 年份:2022 · DOI:10.1149/ma2022-01381656mtgabs

Oxide-based solid-state Li-batteries (SSLiBs) have the potential to be a transformational and intrinsically safe energy storage solution due to their non-flammable ceramic electrolyte that enables the use of high-capacity Li metal anodes and high voltage cathodes for higher energy density over a much wider operating temperature range. However, their progress has been limited due to electrode/electrolyte interfacial issues. In particular for Li-metal anodes concerns over dendrite formation/propagation and the requirement for elevated temperature and high stack pressure are still prevalent. To eliminate these concerns a rational design of tailored structures and interfaces in Li-metal anodes will be presented. In addition, progress toward full cells using these tailored structures and interfaces will be presented.