Facile Synthesis of g-C 3 N 4 /MnO 2 Composites with Dual Functional Activity of Photodegradation of Pollutants and Antimicrobial Efficacy

作者：Paramasivam Shanmugam, Mani Arivazhagan, Alvin Lim Teik Zheng, Lalitha Gnanasekaran, Hongyi Gao, Joon Ching Juan, Pariya Na Nakorn, Supakorn Boonyuen · 发表于：ACS Omega · 年份：2026 · DOI：10.1021/acsomega.5c07860 · 被引用次数：4 · 研究领域：Advanced Photocatalysis Techniques、Advanced oxidation water treatment、TiO2 Photocatalysis and Solar Cells

High Resolution Image Download MS PowerPoint Slide Increasing environmental contamination and spread of drug-resistant microbials leading to water pollution and antimicrobial resistance is a critical issue worldwide. This study describes the synthesis of multifunctional heterojunction g-C 3 N 4 /MnO 2 composite as a potential photocatalyst for environmental remediation and microbial inactivation under visible light. Initially, graphitic carbon nitride (g-C 3 N 4 ) was prepared by a thermal polycondensation method. Further, the multifunctional heterojunction g-C 3 N 4 /MnO 2 composite with uniform MnO 2 nanoparticle (NP) distribution is developed via a simple hydrothermal process. The g-C 3 N 4 /MnO 2 composites were examined through the degradation of tetracycline (TC) and methylene blue (MB). As a result, the composite materials demonstrated superior photocatalytic efficiency than MnO 2 and g-C 3 N 4, due to the composite materials’ enhanced charge separation and extended to the visible light region. Remarkably, degradation efficiencies of 95.38% for MB and 91.97% for TC were achieved within 180 min. Further, antibacterial activity was tested against Escherichia coli and Staphylococcus aureus using the agar–agar well diffusion method. The obtained zone inhibition values reveal that as-prepared g-C 3 N 4 /MnO 2 composites have strong antimicrobial properties. These results demonstrate that g-C 3 N 4 /MnO 2 composites are cost-effective, sustainable, and multifunctional materi...