A hydrogen-bond network sieve enables selective OH − /Cl − discrimination for stable seawater splitting at 2.0 A cm −2

作者：Yang Yu, Wei Zhou, Junshu Yuan, Xiaohan Zhou, Xiaoxiao Meng, Xuewei Zhang, Xuhan Li, Naiyuan Xue, Yingjian Chen, Xia Xiao, Mengyao Gu, Juan Chen, Xingxing Wang, Fei Sun, Jihui Gao, Guangbo Zhao · 发表于：Energy & Environmental Science · 年份：2025 · DOI：10.1039/d5ee04595a · 被引用次数：30 · 研究领域：Advanced Chemical Sensor Technologies、Water Quality Monitoring and Analysis、Mass Spectrometry Techniques and Applications

We established a hydrogen-bond network-mediated ion-sieve for seawater splitting, where selective OH − transport and Cl − exclusion are governed by dynamic interfacial water restructuring, overturning the conventional electrostatic repulsion model.