High Performance Broadband Polarization-Sensitive Photodetector Enabled by Mixed-Dimensional n-ReS 2 /p-GaAs van der Waals Heterostructure

作者：Bing Wang, Pu Zou, Chaoyang Liu, Guoxin Liu, Wanglong Wu, Gaotian Zhang, Zhen Wang, Xiaozhou Wang, Wei Gao, Huaimin Gu, Jingbo Li · 发表于：ACS Applied Materials & Interfaces · 年份：2025 · DOI：10.1021/acsami.5c14804 · 被引用次数：4 · 研究领域：2D Materials and Applications、Photonic and Optical Devices、Nanowire Synthesis and Applications

The realization of photodetectors capable of broadband detection, self-powered operation, and polarization sensitivity is crucial for advancing next-generation optoelectronic technologies. A mixed-dimensional van der Waals heterojunction photodetector composed of two-dimensional ReS 2 and three-dimensional p-type GaAs was designed and fabricated in this study. The device effectively achieves broadband self-powered photodetection across the spectral range of 254–808 nm at zero external bias. When exposed to 365 nm ultraviolet radiation, the photodetector delivers a high responsivity of 0.15 A/W and a specific detectivity reaching 8.39 × 10 11 Jones. Additionally, it demonstrates rapid temporal response, with rise and decay times of 77 and 81 ms, respectively. Benefiting from the intrinsic in-plane anisotropy of the ReS 2 crystal lattice and the effective depletion region at the ReS 2 /GaAs interface, the device reveals pronounced polarization sensitivity, with the polarization ratios of 2.11 at V ds = 0 V and 14.46 at V ds = −1 V under 405 nm. These findings underscore the promising prospects of n-ReS 2 /p-GaAs heterostructures in enabling multifunctional, energy-efficient, and high-performance photodetection, with particular relevance to polarization-resolved imaging and next-generation optical sensing technologies.