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Bioinspired porous Ti2CTX/Si3N4 composites with aligned lamellar structure for efficient microwave absorption

作者:Hailong Xu, Chenyang Jing, Zhijian Xu, Haoyang Zhan, Fang Ye, Qiang Chen, Meng Zhu, Luo Kong, Xinliang Li, Xia Chai, Yuchang Qing, Xiaomeng Fan, Fa Luo · 发表于:Soft Science · 年份:2025 · DOI:10.20517/ss.2025.63 · 被引用次数:35 · 研究领域:MXene and MAX Phase Materials、Electromagnetic wave absorption materials、Boron and Carbon Nanomaterials Research

With the ever-deepening understanding of nano-electromagnetic interactions and the advancements of fabrication methodologies of nanomaterials, diverse electromagnetic platforms utilizing nanomaterials have been developed for next-generation electromagnetic safeguarding applications. This study presents the design and fabrication of bioinspired porous Ti<sub>2</sub>CT<sub>X</sub>/Si<sub>3</sub>N<sub>4</sub> composites featuring an aligned lamellar structure, aimed at facilitating the effective absorption and dissipation of electromagnetic radiation. The layered configuration of Ti<sub>2</sub>CT<sub>X</sub>/Si<sub>3</sub>N<sub>4</sub> composites facilitates the repeated reflection of electromagnetic waves between neighboring Ti<sub>2</sub>CT<sub>X</sub> layers, hence enhancing the energy dissipation of these waves. At a Ti<sub>2</sub>CT<sub>X</sub> concentration of merely 0.21 wt.%, the effective absorption bandwidth of Ti<sub>2</sub>CT<sub>X</sub>/Si<sub>3</sub>N<sub>4</sub> composites encompasses the whole X-band (8.2-12.4 GHz), with a minimum reflection loss of -53 dB achievable at a sample thickness of 5 mm. Simultaneously, the fabricated Ti<sub>2</sub>CT<sub>X</sub>/Si<sub>3</sub>N<sub>4</sub> composites demonstrate advantages in lightwe...