Entanglement of spin transition and structural adaptability: manipulating the slow spin equilibrium by the guest-mediated fine-tuning of elastic frustration

作者：Yuqiao Chai, Yuting Yang, Jin-Peng Xue · 发表于：Chemical Science · 年份：2025 · DOI：10.1039/d5sc01202c · 被引用次数：6 · 研究领域：Quantum many-body systems、Theoretical and Computational Physics、Physics of Superconductivity and Magnetism

↔ HS) processes. In the semi-sealed method, guest molecules gradually escape from the material until the guest-saturated state disappears. This continuous loss shifts the slow spin equilibrium from a state that is difficult to switch to one that fully completes the transition. The study demonstrates that guest molecule modulation is more controllable than structural deformation effects on elastic frustration, offering a pathway to discover hidden types of SCO materials and develop new stimulus-responsive materials.