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Dual-reaction-centre enabled concurrent N–C–N coupling for effective urea electrosynthesis

作者:Junxian Liu, Sean C. Smith, Xin Tan, Yuantong Gu, Liangzhi Kou · 发表于:Journal of Materials Chemistry A · 年份:2025 · DOI:10.1039/d5ta02152a · 被引用次数:9 · 研究领域:Ammonia Synthesis and Nitrogen Reduction、CO2 Reduction Techniques and Catalysts、Covalent Organic Framework Applications

Dual-reaction-centre catalysts PcTM 1 –O 8 –TM 2 facilitate urea electrosynthesis from NO and CO 2 via concurrent N–C–N coupling. The independent reaction centres, TMN 4 and TMO 4 , can be individually optimized for enhanced performance.