Time-Domain-Filtered Terahertz Nanoscopy of Intrinsic Light–Matter Interactions

作者：Xiaoqiuyan Zhang, Xin Zhang, Zhuocheng Zhang, Tianyu Zhang, Xingxing Xu, Fu Tang, Jing Yang, Jiakun Wang, Hui Jiang, Zhaoyun Duan, Yanyu Wei, Yubin Gong, Hui Zhang, Peining Li, Min Hu · 发表于：Nano Letters · 年份：2024 · DOI：10.1021/acs.nanolett.4c03715 · 被引用次数：12 · 研究领域：Terahertz technology and applications、Plasmonic and Surface Plasmon Research、Spectroscopy and Laser Applications

Terahertz (THz) technology holds great potential across diverse applications, including biosensing and information communications, but conventional far-field techniques are limited by diffraction. Near-field optical microscopy overcomes this barrier through a sharp tip that concentrates incident THz waves into nanometric volumes, detecting scattered near-field to reveal nanoscale optical properties. However, owing to the large THz wavelengths, resonant surface waves arising on the tip and cantilever obscure the intrinsic response. Here we combine near-field microscopy with THz time-domain spectroscopy and implement time-domain filtering with an elongated cantilever to eliminate this artifact, achieving intrinsic nanospectroscopy and nanoimaging. By applying this technique, we distinguish and characterize historical pigments of an ancient sculpture, such as vermilion and red lead, on the nanoscale. We also unravel deep-subwavelength localized resonance modes in THz optical antennas, demonstrating capabilities for THz nanophotonics. Our work advances THz nanoimaging and nanospectroscopy techniques to probe intrinsic nanoscale THz light-matter interactions.