Anthropocene 129 I Record in the Yellow Sea Sediments and Its Indication for River-Delivered Radioactive Pollution to Marginal Seas

作者：Yanyun Wang, Tianfeng Guo, Yukun Fan, Luyuan Zhang, Zhigang Guo, Peng Cheng, Jianghu Lan, Qi Liu, Xiaolin Hou · 发表于：Environmental Science & Technology · 年份：2024 · DOI：10.1021/acs.est.4c02123 · 被引用次数：9 · 研究领域：Radioactive contamination and transfer、Isotope Analysis in Ecology、Geology and Paleoclimatology Research

As the number of coastal nuclear facilities rapidly increases and the wastewater from the Fukushima Nuclear Plant has been discharged into the Pacific Ocean, the nuclear environmental safety of China’s marginal seas is gaining increased attention along with the heightened potential risk of nuclear accidents. However, insufficient work limits our understanding of the impact of human nuclear activities on the Yellow Sea (YS) and the assessment of their environmental process. This study first reports the 129 I and 127 I records of posthuman nuclear activities in the two YS sediments. Source identification of anthropogenic 129 I reveals that, in addition to the gaseous 129 I release and re-emission of oceanic 129 I discharged from the European Nuclear Fuel Reprocessing Plants (NFRPs), the Chinese nuclear weapons testing fallout along with the global fallout is an additional 129 I input for the continental shelf of the YS. The 129 I/ 127 I atomic ratios in the North YS (NYS) sediment are significantly higher than those in the other adjacent coastal areas, attributed to the significant riverine input of particulate 129 I by the Yellow River. Furthermore, we found a remarkable 129 I latitudinal disparity in the sediments than those in the seawaters in the various China seas, revealing that sediments in China’s marginal seas already received a huge anthropogenic 129 I from terrigenous sources via rivers and thus became a significant sink of anthropogenic 129 I. This study broadens an...