Size-dependent magnon thermal transport in a nanostructured quantum magnet

作者：Shucheng Guo, Hongze Li, Xue Bai, Yitian Wang, Shuchen Li, Rafal E. Dunin‐Borkowski, Jianshi Zhou, Xi Chen · 发表于：Cell Reports Physical Science · 年份：2024 · DOI：10.1016/j.xcrp.2024.101879 · 被引用次数：9 · 研究领域：Physics of Superconductivity and Magnetism、Quantum and electron transport phenomena、Magnetic properties of thin films

Magnons are fundamental excitations of spin waves in magnetic materials, which are able to carry both heat and spin information. Examining magnon thermal transport is essential for advancing energy-efficient spintronics and novel energy conversion technologies. Unlike the well-established thermal properties of phonons and electrons, the size effect on magnon thermal transport remains elusive. Here, we quantitatively measure the role of grain size on magnon thermal transport in the nanostructured quantum magnet La 2 CuO 4 . Samples with controlled grain sizes are synthesized using a bottom-up method. The measured magnon thermal conductivity decreases as the grain size is reduced. Analysis using a two-dimensional magnon transport kinetic model, combined with optical and electrical measurements, suggests that magnon-boundary scattering effectively restricts the magnon mean free path, suppressing magnon thermal conductivity. These results offer valuable insights into the prediction and control of magnon transport at the nanoscale, especially for applications in quantum information processing and energy conversion.