Local microenvironment tuning induces switching between electrochemical CO 2 reduction pathways

作者：Surani Bin Dolmanan, Annette Böhme, Ziting Fan, Alex J. King, Aidan Q. Fenwick, Albertus D. Handoko, Wan Ru Leow, Adam Z. Weber, Xinbin Ma, Edwin Khoo, Harry A. Atwater, Yanwei Lum · 发表于：Journal of Materials Chemistry A · 年份：2023 · DOI：10.1039/d3ta02558f · 被引用次数：35 · 研究领域：CO2 Reduction Techniques and Catalysts、Ionic liquids properties and applications、Advanced Thermoelectric Materials and Devices

We show that the pore size of the gas-diffusion layer used in electrochemical CO 2 reduction affects CO 2 mass transport. This directly influences the local reaction microenvironment, controlling the selectivity between CO and formate on Ag catalysts.