Pore confined time-of-flight secondary ion electrochemical mass spectrometry

作者：Jun-Gang Wang, Ru‐Jia Yu, Xin Hua, Yi‐Tao Long · 发表于：Chemical Society Reviews · 年份：2023 · DOI：10.1039/d2cs00575a · 被引用次数：28 · 研究领域：Electrochemical Analysis and Applications、Ion-surface interactions and analysis、Electrocatalysts for Energy Conversion

time-of-flight secondary ion electrochemical mass spectrometry with inherent high mass and spatiotemporal resolution has emerged as a promising strategy for investigating electrochemical processes at the electrode surface. This review illustrates the recent advancements in coupling time-of-flight secondary ion mass spectrometry and electrochemistry to visualize and quantify local dynamic electrochemical processes, identify solvated species distribution, and disclose hidden reaction pathways at the molecular level. Moreover, the key challenges in this field are further discussed to promote new applications and discoveries in operando studying the dynamic electrochemical interfaces of advanced energy systems.