In situ performance and stability tests of large-area flexible polymer solar cells in the 35-km stratospheric environment

作者：Zihan Xu, Guoning Xu, Qun Luo, Yunfei Han, Yu Tang, Ying Miao, Yongxiang Li, Jian Qin, Jingbo Guo, Wusong Zha, Chao Gong, Kun Lü, Jianqi Zhang, Zhixiang Wei, Rong Cai, Yanchu Yang, Zhaojie Li, Chang‐Qi Ma · 发表于：National Science Review · 年份：2022 · DOI：10.1093/nsr/nwac285 · 被引用次数：34 · 研究领域：Organic Electronics and Photovoltaics、solar cell performance optimization、Nanowire Synthesis and Applications

ABSTRACT Flexible organic solar cells (FOSCs) are one of the most promising power sources for aerospace aircraft due to their attractive advantages with high power-per-weight ratio and excellent mechanical flexibility. Understanding the performance and stability of high-performance FOSCs is essential for the further development of FOSCs for aerospace applications. In this paper, after systematic investigations on the performance of the state-of-the-art high-performance solar cells under thermal cycle and intensive UV irradiation conditions, in situ performance and stability tests of the solar cells in the 35 km stratospheric environment were carried out through a high-altitude balloon uploading. The encapsulated FOSCs with an area of 0.64 cm2 gave the highest power density of 15.26 mW/cm2 and an efficiency over 11%, corresponding to a power-per-weight ratio of over 3.32 kW/kg. More importantly, the cells showed stable power output during the 3-h continuous flight at 35 km and only 10% performance decay after return to the lab, suggesting promising stability of the FOSCs in the stratospheric environment.