Regulating the interfacial water structure by tensile strain to boost electrochemical semi-hydrogenation of alkynes

作者：Xudong Xu, Jun Ma, Fangfang Wu, Kaili Zhu, Haiqiao Zhou, Ye Zhang, Xiaoyu Li, Yuhu Zhou, Gan Jia, Dong Liu, Peng Gao, Wei Ye · 发表于：Inorganic Chemistry Frontiers · 年份：2022 · DOI：10.1039/d2qi00767c · 被引用次数：32 · 研究领域：Electrocatalysts for Energy Conversion、Advanced Photocatalysis Techniques、Advanced battery technologies research

Interfacial water structure is effectively regulated by tensile strain toward K·H 2 O and 2-HB·H 2 O. K·H 2 O speeds up the ECSH conversion and 2-HB·H 2 O improves the alkene selectivity. PdCu icosahedrons deliver an enhanced the ECSH performance.