Ultra-sensitive flexible Ga2O3 solar-blind photodetector array realized via ultra-thin absorbing medium

作者：Yancheng Chen, Xun Yang, Yuan Zhang, Xuexia Chen, Junlu Sun, Zhiyang Xu, Kaiyong Li, Lin Dong, Chongxin Shan · 发表于：Nano Research · 年份：2021 · DOI：10.1007/s12274-021-3942-6 · 被引用次数：96 · 研究领域：Ga2O3 and related materials、ZnO doping and properties、Transition Metal Oxide Nanomaterials

The quest for solar-blind photodetectors with outstanding optoelectronic properties and weak signals detection capability is essential for their applications in the field of imaging, communication, warning, etc. To date, Ga 2 O 3 has demonstrated potential for high-performance solar-blind photodetectors. However, the performance usually decays superlinearly at low light intensities due to carrier-trapping effect, which limits the weak signal detection capability of Ga 2 O 3 photodetectors. Herein, a Ga 2 O 3 solar-blind photodetector with ultra-thin absorbing medium has been designed to restrain trapping of photo-generated carriers during the transporting process by shortening the carrier transport distance. Meanwhile, multiple-beam interference is employed to enhance the absorption efficiency of the Ga 2 O 3 layer using an Al/Al 2 O 3 /Ga 2 O 3 structure. Based on the ultra-thin absorbing medium with enhanced absorption efficiency, a 7 × 7 flexible photodetector array is developed, and the detectivity can reach 1.7 × 10 15 Jones, which is among the best values ever reported for Ga 2 O 3 photodetectors. Notably, the performance of the photodetector decays little as the illumination intensity is as weak as 5 nW/cm 2 , revealing the capacity to detect ultra-weak signals. In addition, the flexible photodetector array can execute the functions of imaging, spatial distribution of light source intensity, real-time light trajectory detection, etc. Our results may provide a route to ...