Double-Shell and Flower-Like ZnS–C3N4 Derived from in Situ Supramolecular Self-Assembly for Selective Aerobic Oxidation of Amines to Imines

作者：Peng Chen, Linghu Meng, Lang Chen, Jun‐Kang Guo, Sheng Shen, Chak‐Tong Au, Shuang‐Feng Yin · 发表于：ACS Sustainable Chemistry & Engineering · 年份：2019 · DOI：10.1021/acssuschemeng.9b02969 · 被引用次数：54 · 研究领域：Advanced Photocatalysis Techniques、Covalent Organic Framework Applications、Perovskite Materials and Applications

Multishelled micro-/nanostructures have attracted much research attention because of their unique properties. It is a big challenge to fabricate multishelled hollow structures of complex nanoarchitectures with the respective shells different in composition. Herein, the double-shell and flower-like ZnS–C 3 N 4 (2-ZSCN) was fabricated by a facile supramolecular self-assembly method. Because of its unique structure, 2-ZSCN exhibits enhanced photocatalytic activity and stability in the selective aerobic oxidation of amines to imines under visible-light irradiation.