High‐Performance Next‐Generation Perovskite Nanocrystal Scintillator for Nondestructive X‐Ray Imaging

作者：Jin Hyuck Heo, Dong Hee Shin, Jin Kyoung Park, Do Hun Kim, Sang Jin Lee, Sang Hyuk Im · 发表于：Advanced Materials · 年份：2018 · DOI：10.1002/adma.201801743 · 被引用次数：523 · 研究领域：Perovskite Materials and Applications、Luminescence Properties of Advanced Materials、Optical properties and cooling technologies in crystalline materials

Abstract Readily commercializable and cost‐effective next‐generation CsPbBr 3 perovskite nanocrystals (PNCs) based X‐ray detectors are demonstrated. The PNCs‐based X‐ray detector exhibits higher spatial resolution (9.8 lp mm −1 at modulation transfer function (MTF) = 0.2 and 12.5–8.9 lp mm −1 for a linear line chart), faster response time (≈200 ns), and comparable stability (>40 Gy air s −1 of X‐ray exposure) compared with the commercialized terbium‐doped gadolinium oxysulfide (GOS)‐based detectors (spatial resolution = 6.2 lp mm −1 at MTF = 0.2 and 6.3 lp mm −1 for a linear line chart, response time = ≈1200 ns) because the PNCs‐based scintillator has ≈5.6‐fold faster average photoluminescence lifetime and stronger emission than the GOS‐based one.