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Enhanced surface diffusion through termination conversion during epitaxial SrRuO3 growth

作者:Guus Rijnders, Dave H. A. Blank, Jung‐Hoon Choi, Chang‐Beom Eom · 发表于:Applied Physics Letters · 年份:2004 · DOI:10.1063/1.1640472 · 被引用次数:188 · 研究领域:Magnetic and transport properties of perovskites and related materials、Advanced Condensed Matter Physics、Electronic and Structural Properties of Oxides

During the initial growth of the ferromagnetic oxide SrRuO3 on TiO2-terminated SrTiO3, we observe a self-organized conversion of the terminating atomic layer from RuO2 to SrO. This conversion induces an abrupt change in growth mode from layer by layer to growth by step advancement, indicating a large enhancement of the surface diffusivity. This growth mode enables the growth of single-crystalline and single-domain thin films. Both conversion and the resulting growth mode enable the control of the interface properties in heteroepitaxial multilayer structures on an atomic level.